You can legally put down "unemployed" on the LTCF application. There is no requirement that one have a job.
For openly carrying in PA you'll still need a LTCF or a license from any other state to take the firearm in a vehicle whether it is loaded or not. The only way to unlicensed OC in PA is to walk out your front door, and walk to all your destinations.
The only lawful exceptions for transporting in a vehicle in PA is for going to/from: work, place of abode, shooting range, gunsmith, vacation home, or moving from one place of abode to another.
Note also, you will need a LTCF to carry openly in a City of the First Class or during a declared state of emergency.
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