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What I'd really like is some way to calculate theoretical pressures.
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Get and become
proficient with
QuickLoad. I know of no other avenue available to the general public outside of that internal ballistics program.
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...what I'm struggling with is the best propellant to use...
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If you are determined to blow something up,
QuickLoad will quickly show you how..... (I'd also suggest old old truck tire, a long string, a deserted location and a brick wall to stand behind)